Publications associated with Quantum Optoelectronics

Interplay between many body effects and Coulomb screening in the optical bandgap of atomically thin MoS2

Nanoscale Royal Society of Chemistry 9 (2017) 10647-10652

Y Park, SW Han, CCS Chan, BPL Reid, R Taylor, N Kim, Y Jo, H Im, KS Kim

Due to its unique layer-number dependent electronic band structure and strong excitonic features, atomically thin MoS2 is an ideal 2D system where intriguing photoexcited-carrier-induced phenomena can be detected in excitonic luminescence. We perform micro-photoluminescence (PL) measurements and observe that the PL peak redshifts nonlinearly in mono- and bi-layer MoS2 as the excitation power is increased. The excited carrier-induced optical bandgap shrinkage is found to be proportional to n4/3, where n is the optically-induced free carrier density. The large exponent value of 4/3 is explicitly distinguished from a typical value of 1/3 in various semiconductor quantum well systems. The peculiar n4/3 dependent optical bandgap redshift may be due to the interplay between bandgap renormalization and reduced exciton binding energy.

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