Publications


Real-Space Observation of Skyrmionium in a Ferromagnet-Magnetic Topological Insulator Heterostructure.

Nano letters (2018)

S Zhang, F Kronast, G van der Laan, T Hesjedal

The combination of topological insulators, i.e., bulk insulators with gapless, topologically protected surface states, with magnetic order is a love-hate relationship that can unlock new quantum states and exotic physical phenomena, such as the quantum anomalous Hall effect and axion electrodynamics. Moreover, the unusual coupling between topological insulators and ferromagnets can also result in the formation of topological spin textures in the ferromagnetic layer. Skyrmions are topologically-protected magnetization swirls that are promising candidates for spintronics memory carriers. Here, we report on the observation of skyrmionium in thin ferromagnetic films coupled to a magnetic topological insulator. The occurrence of skyrmionium, which appears as a soliton composed of two skyrmions with opposite winding numbers, is tied to the ferromagnetic state of the topological insulator. Our work presents a new combination of two important classes of topological materials and may open the door to new topologically inspired information-storage concepts in the future.


Ab initio calculation of spin fluctuation spectra using time-dependent density functional perturbation theory, plane waves, and pseudopotentials

PHYSICAL REVIEW B 97 (2018) ARTN 024420

K Cao, H Lambert, PG Radaelli, F Giustino

We present an implementation of time-dependent density functional perturbation theory for spin fluctuations, based on plane waves and pseudopotentials. We compute the dynamic spin susceptibility self-consistently by solving the time-dependent Sternheimer equation, within the adiabatic local density approximation to the exchange and correlation kernel. We demonstrate our implementation by calculating the spin susceptibility of representative elemental transition metals, namely bcc Fe, fcc Ni, and bcc Cr. The calculated magnon dispersion relations of Fe and Ni are in agreement with previous work. The calculated spin susceptibility of Cr exhibits a soft-paramagnon instability, indicating the tendency of the Cr spins to condense in an incommensurate spin density wave phase, in agreement with experiment.


Breaking Symmetry with Light: Ultra-Fast Ferroelectricity and Magnetism from Three-Phonon Coupling

Physical review B: Condensed matter and materials physics American Physical Society (2018)

PG Radaelli

A theory describing how ferroic properties can emerge transiently in the ultra-fast regime by breaking symmetry with light through three-phonon coupling is presented. Particular emphasis is placed on the special case when two exactly degenerate mid-infra-red or THz phonons are resonantly pumped, since this situation can give rise to an exactly rectified ferroic response with damping envelopes of ~ 1 ps or less. Light-induced ferroelectricity and ferromagnetism are discussed in this context, and a number of candidate materials that could display these phenomena are proposed. The same analysis is also applied to the interpretation of previous femto-magnetism experiments, performed in different frequency ranges (visible and near-infrared), but sharing similar symmetry characteristics.


Topological surface state of α-Sn on InSb(001) as studied by photoemission

Physical review B: Condensed matter and materials physics American Physical Society 97 (2018) 075101

MR Scholz, L Dudy, F Reis, F Adler, J Aulbach, LJ Collins-McIntyre, LB Duffy, HF Yang, YL Chen, T Hesjedal, ZK Liu, M Hoesch, S Muff, JH Dil, J Schaefer, R Claessen


Magneto-orbital ordering in the divalent A-site quadruple perovskite manganites AMn(7)O(12) (A = Sr, Cd, and Pb)

PHYSICAL REVIEW B 96 (2017) ARTN 054448

RD Johnson, DD Khalyavin, P Manuel, PG Radaelli, IS Glazkova, N Terada, AA Belik


Probing the Topological Surface State in Bi2Se3 Thin Films Using Temperature-Dependent Terahertz Spectroscopy

ACS PHOTONICS 4 (2017) 2711-2718

VS Kamboj, A Singh, T Ferrus, HE Beere, LB Dufry, T Hesjedal, CHW Barnes, DA Ritchie


Codoping of Sb2Te3 thin films with V and Cr

PHYSICAL REVIEW MATERIALS 1 (2017) ARTN 064409

LB Duffy, AI Figueroa, G van der Laan, T Hesjedal


Correction to Step-Flow Growth of Bi 2 Te 3 Nanobelts

Crystal Growth & Design 17 (2017) 1438-1438

P Schönherr, T Tilbury, H Wang, AA Haghighirad, V Srot, PA van Aken, T Hesjedal


Ultrahigh magnetic field spectroscopy reveals the band structure of the three-dimensional topological insulator Bi2Se3

PHYSICAL REVIEW B 96 (2017) ARTN 121111

A Miyata, Z Yang, A Surrente, O Drachenko, DK Maude, O Portugall, LB Duffy, T Hesjedal, P Plochocka, RJ Nicholas


Proposal of a micromagnetic standard problem for ferromagnetic resonance simulations

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 421 (2017) 428-439

A Baker, M Beg, G Ashton, M Albert, D Chernyshenko, W Wang, S Zhang, M-A Bisotti, M Franchin, CL Hu, R Stamps, T Hesjedal, H Fangohr


Deterministic and robust room-temperature exchange coupling in monodomain multiferroic BiFeO3 heterostructures.

Nature communications 8 (2017) 1583-1583

W Saenrang, BA Davidson, F Maccherozzi, JP Podkaminer, J Irwin, RD Johnson, JW Freeland, J Íñiguez, JL Schad, K Reierson, JC Frederick, CAF Vaz, L Howald, TH Kim, S Ryu, MV Veenendaal, PG Radaelli, SS Dhesi, MS Rzchowski, CB Eom

Exploiting multiferroic BiFeO3 thin films in spintronic devices requires deterministic and robust control of both internal magnetoelectric coupling in BiFeO3, as well as exchange coupling of its antiferromagnetic order to a ferromagnetic overlayer. Previous reports utilized approaches based on multi-step ferroelectric switching with multiple ferroelectric domains. Because domain walls can be responsible for fatigue, contain localized charges intrinsically or via defects, and present problems for device reproducibility and scaling, an alternative approach using a monodomain magnetoelectric state with single-step switching is desirable. Here we demonstrate room temperature, deterministic and robust, exchange coupling between monodomain BiFeO3 films and Co overlayer that is intrinsic (i.e., not dependent on domain walls). Direct coupling between BiFeO3 antiferromagnetic order and Co magnetization is observed, with ~ 90° in-plane Co moment rotation upon single-step switching that is reproducible for hundreds of cycles. This has important consequences for practical, low power non-volatile magnetoelectric devices utilizing BiFeO3.


Proposal of a micromagnetic standard problem for ferromagnetic resonance simulations

Journal of Magnetism and Magnetic Materials 421 (2017) 428

AA Baker, M Beg, G Ashton, M Albert, D Chernyshenko, W Wang, S Zhang, M-A Bisotti, M Franchin, CL Hu, R Stamps, T Hesjedal, H Fangohr

Nowadays, micromagnetic simulations are a common tool for studying a wide range of different magnetic phenomena, including the ferromagnetic resonance. A technique for evaluating reliability and validity of different micromagnetic simulation tools is the simulation of proposed standard problems. We propose a new standard problem by providing a detailed specification and analysis of a sufficiently simple problem. By analyzing the magnetization dynamics in a thin permalloy square sample, triggered by a well defined excitation, we obtain the ferromagnetic resonance spectrum and identify the resonance modes via Fourier transform. Simulations are performed using both finite difference and finite element numerical methods, with OOMMF and Nmag simulators, respectively. We report the effects of initial conditions and simulation parameters on the character of the observed resonance modes for this standard problem. We provide detailed instructions and code to assist in using the results for evaluation of new simulator tools, and to help with numerical calculation of ferromagnetic resonance spectra and modes in general.


Synthesis of Superconductor-Topological Insulator Hybrid Nanoribbon Structures

NANO 12 (2017) ARTN 1750095

P Schonherr, F Zhang, V Srot, P van Aken, T Hesjedal


Room-temperature helimagnetism in FeGe thin films.

Scientific reports 7 (2017) 123-

SL Zhang, I Stasinopoulos, T Lancaster, F Xiao, A Bauer, F Rucker, AA Baker, AI Figueroa, Z Salman, FL Pratt, SJ Blundell, T Prokscha, A Suter, J Waizner, M Garst, D Grundler, G van der Laan, C Pfleiderer, T Hesjedal

Chiral magnets are promising materials for the realisation of high-density and low-power spintronic memory devices. For these future applications, a key requirement is the synthesis of appropriate materials in the form of thin films ordering well above room temperature. Driven by the Dzyaloshinskii-Moriya interaction, the cubic compound FeGe exhibits helimagnetism with a relatively high transition temperature of 278 K in bulk crystals. We demonstrate that this temperature can be enhanced significantly in thin films. Using x-ray scattering and ferromagnetic resonance techniques, we provide unambiguous experimental evidence for long-wavelength helimagnetic order at room temperature and magnetic properties similar to the bulk material. We obtain α intr = 0.0036 ± 0.0003 at 310 K for the intrinsic damping parameter. We probe the dynamics of the system by means of muon-spin rotation, indicating that the ground state is reached via a freezing out of slow dynamics. Our work paves the way towards the fabrication of thin films of chiral magnets that host certain spin whirls, so-called skyrmions, at room temperature and potentially offer integrability into modern electronics.


X-ray magnetic circular dichroism study of Dy-doped Bi2Te3 topological insulator thin films

JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 422 (2017) 93-99

AI Figueroa, AA Baker, SE Harrison, K Kummer, G van der Laan, T Hesjedal


Direct experimental determination of spiral spin structures via the dichroism extinction effect in resonant elastic soft x-ray scattering

PHYSICAL REVIEW B 96 (2017) ARTN 094401

SL Zhang, G van der Laan, T Hesjedal


Perfect quintuple layer Bi2Te3 nanowires: Growth and thermoelectric properties

APL MATERIALS 5 (2017) ARTN 086110

P Schonherr, D Kojda, V Srot, SF Fischer, PA van Aken, T Hesjedal


Magnetic proximity coupling to Cr-doped Sb2Te3 thin films

PHYSICAL REVIEW B 95 (2017) ARTN 224422

LB Duffy, AI Figueroa, L Gladczuk, N-J Steinke, K Kummer, G van der Laan, T Hesjedal


Strain and Magnetic Field Induced Spin-Structure Transitions in Multiferroic BiFeO3

ADVANCED MATERIALS 29 (2017) UNSP 1602327

A Agbelele, D Sando, C Toulouse, C Paillard, RD Johnson, R Ruffer, AF Popkov, C Carretero, P Rovillain, J-M Le Breton, B Dkhil, M Cazayous, Y Gallais, M-A Measson, A Sacuto, P Manuel, AK Zvezdin, A Barthelemy, J Juraszek, M Bibes


Emergence of Dirac-like bands in the monolayer limit of epitaxial Ge films on Au(1 1 1)

2D Materials 4 (2017) 031005

NBM Schröter, MD Watson, LB Duffy, M Hoesch, Y Chen, T Hesjedal, TK Kim

After the discovery of Dirac fermions in graphene, it has become a natural question to ask whether it is possible to realize Dirac fermions in other two-dimensional (2D) materials as well. In this work, we report the discovery of multiple Dirac-like electronic bands in ultrathin Ge flms grown on Au(1 1 1) by angle-resolved photoelectron spectroscopy. By tuning the thickness of the flms, we are able to observe the evolution of their electronic structure when passing through the monolayer limit. Our discovery may signify the synthesis of germanene, a 2D honeycomb structure made of Ge, which is a promising platform for exploring exotic topological phenomena and enabling potential applications.

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