Focal aberrations of large-aperture HOPG von-Hàmos x-ray spectrometers

Journal of Instrumentation 7 (2012)

U Zastrau, CRD Brown, T Döppner, SH Glenzer, G Gregori, HJ Lee, H Marschner, S Toleikis, O Wehrhan, E Förster

Focal aberrations of large-aperture highly oriented pyrolytic graphite (HOPG) crystals in von-Hàmos geometry are investigated by experimental and computational methods. A mosaic HOPG crystal film of 100 μm thickness diffracts 8 keV x-rays. This thickness is smaller than the absorption depth of the symmetric 004-reflection, which amounts to 257 μm. Cylindrically bent crystals with 110mm radius of curvature and up to 100 mm collection width produce a X-shaped halo around the focus. This feature vanishes when the collection aperture is reduced, but axial spectral profiles show that the resolution is not affected. X-ray topography reveals significant inhomogeneous crystallite domains of 2±1mm diameter along the entire crystal. Rocking curves shift by about ±20arcmin between domains, while their full width at half-maximum varies between 30 and 50 arcmin. These inhomogeneities are not imprinted at the focal spot, since the monochromatically reflecting area of the crystal is large compared to inhomogeneities. Ray-tracing calculations using a Monte-Carlo-based algorithm developed for mosaic crystals reproduce the X-shaped halo in the focal plane, stemming from the mosaic defocussing in the non-dispersive direction in combination with large apertures. The best achievable resolution is found by analyzing a diversity of rocking curve widths, source sizes and crystal thicknesses for 8 keV x-rays to be ΔE/E ∼ 10 -4 . Finally a general analytic expression for the shape of the aberration is derived. © 2012 IOP Publishing Ltd and Sissa Medialab srl.

Direct measurements of the ionization potential depression in a dense plasma

Physical Review Letters 109 (2012)

O Ciricosta, SM Vinko, HK Chung, BI Cho, CRD Brown, T Burian, J Chalupský, K Engelhorn, RW Falcone, C Graves, V Hájková, A Higginbotham, L Juha, J Krzywinski, HJ Lee, M Messerschmidt, CD Murphy, Y Ping, DS Rackstraw, A Scherz, W Schlotter, S Toleikis, JJ Turner, L Vysin, T Wang, B Wu, U Zastrau, D Zhu, RW Lee, P Heimann, B Nagler, JS Wark

We have used the Linac Coherent Light Source to generate solid-density aluminum plasmas at temperatures of up to 180 eV. By varying the photon energy of the x rays that both create and probe the plasma, and observing the K-α fluorescence, we can directly measure the position of the K edge of the highly charged ions within the system. The results are found to disagree with the predictions of the extensively used Stewart-Pyatt model, but are consistent with the earlier model of Ecker and Kröll, which predicts significantly greater depression of the ionization potential. © 2012 American Physical Society.

Inelastic x-ray scattering from shocked liquid deuterium

Physical Review Letters 109 (2012)

SP Regan, K Falk, G Gregori, PB Radha, SX Hu, TR Boehly, BJB Crowley, SH Glenzer, OL Landen, DO Gericke, T Döppner, DD Meyerhofer, CD Murphy, TC Sangster, J Vorberger

The Fermi-degenerate plasma conditions created in liquid deuterium by a laser-ablation - driven shock wave were probed with noncollective, spectrally resolved, inelastic x-ray Thomson scattering employing Cl Ly α line emission at 2.96 keV. These first x-ray Thomson scattering measurements of the microscopic properties of shocked deuterium show an inferred spatially averaged electron temperature of 8±5 eV, an electron density of 2.2(±0.5)×1023 cm - 3, and an ionization of 0.8 (-0.25, +0.15). Two-dimensional hydrodynamic simulations using equation-of-state models suited for the extreme parameters occurring in inertial confinement fusion research and planetary interiors are consistent with the experimental results. © 2012 American Physical Society.

Molecular Dynamics Simulations for the Shear Viscosity of the One-Component Plasma


JP Mithen, J Daligault, G Gregori

Warm Dense Aluminum Plasma generated by the Free-Electron-Laser FLASH


U Zastrau, SM Vinko, JS Wark, S Toleikis, T Tschentscher, SH Glenzer, RW Lee, AJ Nelson, TWJ Dzelzainis, D Riley, B Nagler, E Galtier, FB Rosmej, E Foerster

Creation and diagnosis of a solid-density plasma with an X-ray free-electron laser.

Nature 482 (2012) 59-62

SM Vinko, O Ciricosta, BI Cho, K Engelhorn, H-K Chung, CRD Brown, T Burian, J Chalupský, RW Falcone, C Graves, V Hájková, A Higginbotham, L Juha, J Krzywinski, HJ Lee, M Messerschmidt, CD Murphy, Y Ping, A Scherz, W Schlotter, S Toleikis, JJ Turner, L Vysin, T Wang, B Wu, U Zastrau, D Zhu, RW Lee, PA Heimann, B Nagler, JS Wark

Matter with a high energy density (>10(5) joules per cm(3)) is prevalent throughout the Universe, being present in all types of stars and towards the centre of the giant planets; it is also relevant for inertial confinement fusion. Its thermodynamic and transport properties are challenging to measure, requiring the creation of sufficiently long-lived samples at homogeneous temperatures and densities. With the advent of the Linac Coherent Light Source (LCLS) X-ray laser, high-intensity radiation (>10(17) watts per cm(2), previously the domain of optical lasers) can be produced at X-ray wavelengths. The interaction of single atoms with such intense X-rays has recently been investigated. An understanding of the contrasting case of intense X-ray interaction with dense systems is important from a fundamental viewpoint and for applications. Here we report the experimental creation of a solid-density plasma at temperatures in excess of 10(6) kelvin on inertial-confinement timescales using an X-ray free-electron laser. We discuss the pertinent physics of the intense X-ray-matter interactions, and illustrate the importance of electron-ion collisions. Detailed simulations of the interaction process conducted with a radiative-collisional code show good qualitative agreement with the experimental results. We obtain insights into the evolution of the charge state distribution of the system, the electron density and temperature, and the timescales of collisional processes. Our results should inform future high-intensity X-ray experiments involving dense samples, such as X-ray diffractive imaging of biological systems, material science investigations, and the study of matter in extreme conditions.

Resonant Kα spectroscopy of solid-density aluminum plasmas

Physical Review Letters 109 (2012)

BI Cho, K Engelhorn, SM Vinko, HK Chung, O Ciricosta, DS Rackstraw, RW Falcone, CRD Brown, T Burian, J Chalupský, C Graves, V Hájková, A Higginbotham, L Juha, J Krzywinski, HJ Lee, M Messersmidt, C Murphy, Y Ping, N Rohringer, A Scherz, W Schlotter, S Toleikis, JJ Turner, L Vysin, T Wang, B Wu, U Zastrau, D Zhu, RW Lee, B Nagler, JS Wark, PA Heimann

The x-ray intensities made available by x-ray free electron lasers (FEL) open up new x-ray matter interaction channels not accessible with previous sources. We report here on the resonant generation of Kα emission, that is to say the production of copious Kα radiation by tuning the x-ray FEL pulse to photon energies below that of the K edge of a solid aluminum sample. The sequential absorption of multiple photons in the same atom during the 80 fs pulse, with photons creating L-shell holes and then one resonantly exciting a K-shell electron into one of these holes, opens up a channel for the Kα production, as well as the absorption of further photons. We demonstrate rich spectra of such channels, and investigate the emission produced by tuning the FEL energy to the K-L transitions of those highly charged ions that have transition energies below the K edge of the cold material. The spectra are sensitive to x-ray intensity dependent opacity effects, with ions containing L-shell holes readily reabsorbing the Kα radiation. © 2012 American Physical Society.

Self-organized electromagnetic field structures in laser-produced counter-streaming plasmas

Nature Physics 8 (2012) 809-812

NL Kugland, DD Ryutov, PY Chang, RP Drake, G Fiksel, DH Froula, SH Glenzer, G Gregori, M Grosskopf, M Koenig, Y Kuramitsu, C Kuranz, MC Levy, E Liang, J Meinecke, F Miniati, T Morita, A Pelka, C Plechaty, R Presura, A Ravasio, BA Remington, B Reville, JS Ross, Y Sakawa, A Spitkovsky, H Takabe, HS Park

Self-organization occurs in plasmas when energy progressively transfers from smaller to larger scales in an inverse cascade. Global structures that emerge from turbulent plasmas can be found in the laboratory and in astrophysical settings; for example, the cosmic magnetic field, collisionless shocks in supernova remnants and the internal structures of newly formed stars known as Herbig-Haro objects. Here we show that large, stable electromagnetic field structures can also arise within counter-streaming supersonic plasmas in the laboratory. These surprising structures, formed by a yet unexplained mechanism, are predominantly oriented transverse to the primary flow direction, extend for much larger distances than the intrinsic plasma spatial scales and persist for much longer than the plasma kinetic timescales. Our results challenge existing models of counter-streaming plasmas and can be used to better understand large-scale and long-time plasma self-organization. © 2012 Macmillan Publishers Limited. All rights reserved.

Measuring electron-positron annihilation radiation from laser plasma interactions

Review of Scientific Instruments 83 (2012)

H Chen, R Tommasini, J Seely, CI Szabo, U Feldman, N Pereira, G Gregori, K Falk, J Mithen, CD Murphy

We investigated various diagnostic techniques to measure the 511 keV annihilation radiations. These include step-wedge filters, transmission crystal spectroscopy, single-hit CCD detectors, and s treaked scintillating detection. While none of the diagnostics recorded conclusive results, the step-wedge filter that is sensitive to the energy range between 100 keV and 700 keV shows a signal around 500 keV that is clearly departing from a pure Bremsstrahlung spectrum and that we ascribe to annihilation radiation. © 2012 American Institute of Physics.

Laboratory investigations on the origins of cosmic rays

Plasma Physics and Controlled Fusion 54 (2012)

Y Kuramitsu, Y Sakawa, T Morita, T Ide, K Nishio, H Tanji, H Aoki, S Dono, CD Gregory, JN Waugh, N Woolsey, A Dizière, A Pelka, A Ravasio, B Loupias, M Koenig, SA Pikuz, YT Li, Y Zhang, X Liu, JY Zhong, J Zhang, G Gregori, N Nakanii, K Kondo, Y Mori, E Miura, R Kodama, Y Kitagawa, K Mima, KA Tanaka, H Azechi, T Moritaka, Y Matsumoto, T Sano, A Mizuta, N Ohnishi, M Hoshino, H Takabe

We report our recent efforts on the experimental investigations related to the origins of cosmic rays. The origins of cosmic rays are long standing open issues in astrophysics. The galactic and extragalactic cosmic rays are considered to be accelerated in non-relativistic and relativistic collisionless shocks in the universe, respectively. However, the acceleration and transport processes of the cosmic rays are not well understood, and how the collisionless shocks are created is still under investigation. Recent high-power and high-intensity laser technologies allow us to simulate astrophysical phenomena in laboratories. We present our experimental results of collisionless shock formations in laser-produced plasmas. © 2012 IOP Publishing Ltd.

Nanosecond white-light Laue diffraction measurements of dislocation microstructure in shock-compressed single-crystal copper.

Nat Commun 3 (2012) 1224-

MJ Suggit, A Higginbotham, JA Hawreliak, G Mogni, G Kimminau, P Dunne, AJ Comley, N Park, BA Remington, JS Wark

Under uniaxial high-stress shock compression it is believed that crystalline materials undergo complex, rapid, micro-structural changes to relieve the large applied shear stresses. Diagnosing the underlying mechanisms involved remains a significant challenge in the field of shock physics, and is critical for furthering our understanding of the fundamental lattice-level physics, and for the validation of multi-scale models of shock compression. Here we employ white-light X-ray Laue diffraction on a nanosecond timescale to make the first in situ observations of the stress relaxation mechanism in a laser-shocked crystal. The measurements were made on single-crystal copper, shocked along the [001] axis to peak stresses of order 50 GPa. The results demonstrate the presence of stress-dependent lattice rotations along specific crystallographic directions. The orientation of the rotations suggests that there is double slip on conjugate systems. In this model, the rotation magnitudes are consistent with defect densities of order 10(12) cm(-2).

Studying astrophysical collisionless shocks with counterstreaming plasmas from high power lasers

High Energy Density Physics 8 (2012) 38-45

HS Park, DD Ryutov, JS Ross, NL Kugland, SH Glenzer, C Plechaty, SM Pollaine, BA Remington, A Spitkovsky, L Gargate, G Gregori, A Bell, C Murphy, Y Sakawa, Y Kuramitsu, T Morita, H Takabe, DH Froula, G Fiksel, F Miniati, M Koenig, A Ravasio, A Pelka, E Liang, N Woolsey, CC Kuranz, RP Drake, MJ Grosskopf

Collisions of high Mach number flows occur frequently in astrophysics, and the resulting shock waves are responsible for the properties of many astrophysical phenomena, such as supernova remnants, Gamma Ray Bursts and jets from Active Galactic Nuclei. Because of the low density of astrophysical plasmas, the mean free path due to Coulomb collisions is typically very large. Therefore, most shock waves in astrophysics are "collisionless", since they form due to plasma instabilities and self-generated magnetic fields. Laboratory experiments at the laser facilities can achieve the conditions necessary for the formation of collisionless shocks, and will provide a unique avenue for studying the nonlinear physics of collisionless shock waves. We are performing a series of experiments at the Omega and Omega-EP lasers, in Rochester, NY, with the goal of generating collisionless shock conditions by the collision of two high-speed plasma flows resulting from laser ablation of solid targets using ∼10 16 W/cm 2 laser irradiation. The experiments will aim to answer several questions of relevance to collisionless shock physics: the importance of the electromagnetic filamentation (Weibel) instabilities in shock formation, the self-generation of magnetic fields in shocks, the influence of external magnetic fields on shock formation, and the signatures of particle acceleration in shocks. Our first experiments using Thomson scattering diagnostics studied the plasma state from a single foil and from double foils whose flows collide "head-on" Our data showed that the flow velocity and electron density were 10 8 cm/s and 10 19 cm -3 , respectively, where the Coulomb mean free path is much larger than the size of the interaction region. Simulations of our experimental conditions show that weak Weibel mediated current filamentation and magnetic field generation were likely starting to occur. This paper presents the results from these first Omega experiments. © 2011.

Self-consistent measurement of the equation of state of liquid deuterium


K Falk, SP Regan, J Vorberger, MA Barrios, TR Boehly, DE Fratanduono, SH Glenzer, DG Hicks, SX Hu, CD Murphy, PB Radha, S Rothman, AP Jephcoat, JS Watt, DO Gericke, G Gregori

Design considerations for unmagnetized collisionless-shock measurements in homologous flows

Astrophysical Journal 749 (2012)

RP Drake, G Gregori

The subject of this paper is the design of practical laser experiments that can produce collisionless shocks mediated by the Weibel instability. Such shocks may be important in a wide range of astrophysical systems. Three issues are considered. The first issue is the implications of the fact that such experiments will produce expanding flows that are approximately homologous. As a result, both the velocity and the density of the interpenetrating plasma streams will be time dependent. The second issue is the implications of the linear theory of the Weibel instability. For the experiments, the instability is in a regime where standard simplifications do not apply. It appears feasible but non-trivial to obtain adequate growth. The third issue is collisionality. The need to keep resistive magnetic-field dissipation small enough implies that the plasmas should not be allowed to cool substantially. © 2012. The American Astronomical Society. All rights reserved.

Measurement of radiative shock properties by X-ray Thomson scattering

Physical Review Letters 108 (2012)

AJ Visco, RP Drake, SH Glenzer, T Döppner, G Gregori, DH Froula, MJ Grosskopf

X-ray Thomson scattering has enabled us to measure the temperature of a shocked layer, produced in the laboratory, that is relevant to shocks emerging from supernovas. High energy lasers are used to create a shock in argon gas which is probed by x-ray scattering. The scattered, inelastic Compton feature allows inference of the electron temperature. It is measured to be 34 eV in the radiative precursor and ∼60eV near the shock. Comparison of energy fluxes implied by the data demonstrates that the shock wave is strongly radiative. © 2012 American Physical Society.

Testing quantum mechanics in non-Minkowski space-time with high power lasers and 4 th generation light sources

Scientific Reports 2 (2012)

BJB Crowley, R Bingham, RG Evans, DO Gericke, OL Landen, CD Murphy, PA Norreys, SJ Rose, T Tschentscher, CHT Wang, JS Wark, G Gregori

A common misperception of quantum gravity is that it requires accessing energies up to the Planck scale of 10 19 GeV, which is unattainable from any conceivable particle collider. Thanks to the development of ultra-high intensity optical lasers, very large accelerations can be now the reached at their focal spot, thus mimicking, by virtue of the equivalence principle, a non Minkowski space-time. Here we derive a semiclassical extension of quantum mechanics that applies to different metrics, but under the assumption of weak gravity. We use our results to show that Thomson scattering of photons by uniformly accelerated electrons predicts an observable effect depending upon acceleration and local metric. In the laboratory frame, a broadening of the Thomson scattered x ray light from a fourth generation light source can be used to detect the modification of the metric associated to electrons accelerated in the field of a high power optical laser.

X-ray Thomson scattering on shocked graphite

High Energy Density Physics 8 (2012) 46-49

D Kraus, A Otten, A Frank, V Bagnoud, A Blažević, DO Gericke, G Gregori, A Ortner, G Schaumann, D Schumacher, J Vorberger, F Wagner, K Wünsch, M Roth

We present measurements of the changes in the microscopic structure of graphite in a laser-driven shock experiment with X-ray scattering. Laser radiation with intensities of ∼2 × 10 13 W/cm 2 compressed the carbon samples by a factor of two reaching pressures of ∼90 GPa. Due to the change of the crystalline structure the scattered signals of the probe radiation were modified significantly in intensity and spectral composition compared to the scattering on cold samples. It is shown that the elastic scattering on tightly bound electrons increases strongly due to the phase transition whereas the inelastic scattering on weakly bound electrons remains nearly unchanged for the chosen geometry. © 2011 Elsevier B.V.

Observation of inhibited electron-ion coupling in strongly heated graphite.

Sci Rep 2 (2012) 889-

TG White, J Vorberger, CRD Brown, BJB Crowley, P Davis, SH Glenzer, JWO Harris, DC Hochhaus, S Le Pape, T Ma, CD Murphy, P Neumayer, LK Pattison, S Richardson, DO Gericke, G Gregori

Creating non-equilibrium states of matter with highly unequal electron and lattice temperatures (T(ele)≠T(ion)) allows unsurpassed insight into the dynamic coupling between electrons and ions through time-resolved energy relaxation measurements. Recent studies on low-temperature laser-heated graphite suggest a complex energy exchange when compared to other materials. To avoid problems related to surface preparation, crystal quality and poor understanding of the energy deposition and transport mechanisms, we apply a different energy deposition mechanism, via laser-accelerated protons, to isochorically and non-radiatively heat macroscopic graphite samples up to temperatures close to the melting threshold. Using time-resolved x ray diffraction, we show clear evidence of a very small electron-ion energy transfer, yielding approximately three times longer relaxation times than previously reported. This is indicative of the existence of an energy transfer bottleneck in non-equilibrium warm dense matter.

Molecular dynamics simulations of ramp-compressed copper

PHYSICAL REVIEW B 85 (2012) ARTN 024112

A Higginbotham, J Hawreliak, EM Bringa, G Kimminau, N Park, E Reed, BA Remington, JS Wark

Generation of scaled protogalactic seed magnetic fields in laser-produced shock waves.

Nature 481 (2012) 480-483

G Gregori, A Ravasio, CD Murphy, K Schaar, A Baird, AR Bell, A Benuzzi-Mounaix, R Bingham, C Constantin, RP Drake, M Edwards, ET Everson, CD Gregory, Y Kuramitsu, W Lau, J Mithen, C Niemann, H-S Park, BA Remington, B Reville, APL Robinson, DD Ryutov, Y Sakawa, S Yang, NC Woolsey, M Koenig, F Miniati

The standard model for the origin of galactic magnetic fields is through the amplification of seed fields via dynamo or turbulent processes to the level consistent with present observations. Although other mechanisms may also operate, currents from misaligned pressure and temperature gradients (the Biermann battery process) inevitably accompany the formation of galaxies in the absence of a primordial field. Driven by geometrical asymmetries in shocks associated with the collapse of protogalactic structures, the Biermann battery is believed to generate tiny seed fields to a level of about 10(-21) gauss (refs 7, 8). With the advent of high-power laser systems in the past two decades, a new area of research has opened in which, using simple scaling relations, astrophysical environments can effectively be reproduced in the laboratory. Here we report the results of an experiment that produced seed magnetic fields by the Biermann battery effect. We show that these results can be scaled to the intergalactic medium, where turbulence, acting on timescales of around 700 million years, can amplify the seed fields sufficiently to affect galaxy evolution.