Nanosecond white-light Laue diffraction measurements of dislocation microstructure in shock-compressed single-crystal copper.
Nat Commun 3 (2012) 1224-
Under uniaxial high-stress shock compression it is believed that crystalline materials undergo complex, rapid, micro-structural changes to relieve the large applied shear stresses. Diagnosing the underlying mechanisms involved remains a significant challenge in the field of shock physics, and is critical for furthering our understanding of the fundamental lattice-level physics, and for the validation of multi-scale models of shock compression. Here we employ white-light X-ray Laue diffraction on a nanosecond timescale to make the first in situ observations of the stress relaxation mechanism in a laser-shocked crystal. The measurements were made on single-crystal copper, shocked along the  axis to peak stresses of order 50 GPa. The results demonstrate the presence of stress-dependent lattice rotations along specific crystallographic directions. The orientation of the rotations suggests that there is double slip on conjugate systems. In this model, the rotation magnitudes are consistent with defect densities of order 10(12) cm(-2).
Journal of Instrumentation 7 (2012)
Focal aberrations of large-aperture highly oriented pyrolytic graphite (HOPG) crystals in von-Hàmos geometry are investigated by experimental and computational methods. A mosaic HOPG crystal film of 100 μm thickness diffracts 8 keV x-rays. This thickness is smaller than the absorption depth of the symmetric 004-reflection, which amounts to 257 μm. Cylindrically bent crystals with 110mm radius of curvature and up to 100 mm collection width produce a X-shaped halo around the focus. This feature vanishes when the collection aperture is reduced, but axial spectral profiles show that the resolution is not affected. X-ray topography reveals significant inhomogeneous crystallite domains of 2±1mm diameter along the entire crystal. Rocking curves shift by about ±20arcmin between domains, while their full width at half-maximum varies between 30 and 50 arcmin. These inhomogeneities are not imprinted at the focal spot, since the monochromatically reflecting area of the crystal is large compared to inhomogeneities. Ray-tracing calculations using a Monte-Carlo-based algorithm developed for mosaic crystals reproduce the X-shaped halo in the focal plane, stemming from the mosaic defocussing in the non-dispersive direction in combination with large apertures. The best achievable resolution is found by analyzing a diversity of rocking curve widths, source sizes and crystal thicknesses for 8 keV x-rays to be ΔE/E ∼ 10-4. Finally a general analytic expression for the shape of the aberration is derived. © 2012 IOP Publishing Ltd and Sissa Medialab srl.
Energy transport in short-pulse-laser-heated targets measured using extreme ultraviolet laser backlighting
Physical Review E 86 (2012)
High Energy Density Physics 8 (2012) 307-312
Physical Review Letters 109 (2012)
The x-ray intensities made available by x-ray free electron lasers (FEL) open up new x-ray matter interaction channels not accessible with previous sources. We report here on the resonant generation of Kα emission, that is to say the production of copious Kα radiation by tuning the x-ray FEL pulse to photon energies below that of the K edge of a solid aluminum sample. The sequential absorption of multiple photons in the same atom during the 80 fs pulse, with photons creating L-shell holes and then one resonantly exciting a K-shell electron into one of these holes, opens up a channel for the Kα production, as well as the absorption of further photons. We demonstrate rich spectra of such channels, and investigate the emission produced by tuning the FEL energy to the K-L transitions of those highly charged ions that have transition energies below the K edge of the cold material. The spectra are sensitive to x-ray intensity dependent opacity effects, with ions containing L-shell holes readily reabsorbing the Kα radiation. © 2012 American Physical Society.
39th EPS Conference on Plasma Physics 2012, EPS 2012 and the 16th International Congress on Plasma Physics 2 (2012) 938-941
Review of Scientific Instruments 83 (2012)
We investigated various diagnostic techniques to measure the 511 keV annihilation radiations. These include step-wedge filters, transmission crystal spectroscopy, single-hit CCD detectors, and streaked scintillating detection. While none of the diagnostics recorded conclusive results, the step-wedge filter that is sensitive to the energy range between 100 keV and 700 keV shows a signal around 500 keV that is clearly departing from a pure Bremsstrahlung spectrum and that we ascribe to annihilation radiation. © 2012 American Institute of Physics.
High Energy Density Physics 8 (2012) 46-49
We present measurements of the changes in the microscopic structure of graphite in a laser-driven shock experiment with X-ray scattering. Laser radiation with intensities of ∼2 × 10 13 W/cm 2 compressed the carbon samples by a factor of two reaching pressures of ∼90 GPa. Due to the change of the crystalline structure the scattered signals of the probe radiation were modified significantly in intensity and spectral composition compared to the scattering on cold samples. It is shown that the elastic scattering on tightly bound electrons increases strongly due to the phase transition whereas the inelastic scattering on weakly bound electrons remains nearly unchanged for the chosen geometry. © 2011 Elsevier B.V.
CONTRIBUTIONS TO PLASMA PHYSICS 52 (2012) 58-61
Revealing multiphoton resonant ionization in solid density plasmas with an x-ray free electron laser
2012 Conference on Lasers and Electro-Optics, CLEO 2012 (2012)
Interaction of intense x-ray and solid density Al plasma is studied via K-shell emission spectroscopy. A high fluence, high-intensity x-ray pulse from an x-ray free-electron laser unveils multiphoton ionization pathway and drives hidden resonances. © 2012 OSA.
AIP Conference Proceedings 1426 (2012) 975-978
The lattice level strain measured using in situ x-ray diffraction during shock compression of rolled iron foils is used along with the pressure dependent elastic constants to estimate the dynamic strength of 1±1 GPa at 15 GPa. We examine these results in the context of the constant stress (Voigt) and constant strain (Ruess) limit of grain interaction, discussing the implications at the lattice level. © 2012 American Institute of Physics.
Nature Physics (2012)
Nature Physics 8 (2012) 809-812
Self-organization occurs in plasmas when energy progressively transfers from smaller to larger scales in an inverse cascade. Global structures that emerge from turbulent plasmas can be found in the laboratory and in astrophysical settings; for example, the cosmic magnetic field, collisionless shocks in supernova remnants and the internal structures of newly formed stars known as Herbig-Haro objects. Here we show that large, stable electromagnetic field structures can also arise within counter-streaming supersonic plasmas in the laboratory. These surprising structures, formed by a yet unexplained mechanism, are predominantly oriented transverse to the primary flow direction, extend for much larger distances than the intrinsic plasma spatial scales and persist for much longer than the plasma kinetic timescales. Our results challenge existing models of counter-streaming plasmas and can be used to better understand large-scale and long-time plasma self-organization. © 2012 Macmillan Publishers Limited. All rights reserved.
High Energy Density Physics 8 (2012) 38-45
Collisions of high Mach number flows occur frequently in astrophysics, and the resulting shock waves are responsible for the properties of many astrophysical phenomena, such as supernova remnants, Gamma Ray Bursts and jets from Active Galactic Nuclei. Because of the low density of astrophysical plasmas, the mean free path due to Coulomb collisions is typically very large. Therefore, most shock waves in astrophysics are "collisionless", since they form due to plasma instabilities and self-generated magnetic fields. Laboratory experiments at the laser facilities can achieve the conditions necessary for the formation of collisionless shocks, and will provide a unique avenue for studying the nonlinear physics of collisionless shock waves. We are performing a series of experiments at the Omega and Omega-EP lasers, in Rochester, NY, with the goal of generating collisionless shock conditions by the collision of two high-speed plasma flows resulting from laser ablation of solid targets using ∼10 16 W/cm 2 laser irradiation. The experiments will aim to answer several questions of relevance to collisionless shock physics: the importance of the electromagnetic filamentation (Weibel) instabilities in shock formation, the self-generation of magnetic fields in shocks, the influence of external magnetic fields on shock formation, and the signatures of particle acceleration in shocks. Our first experiments using Thomson scattering diagnostics studied the plasma state from a single foil and from double foils whose flows collide "head-on" Our data showed that the flow velocity and electron density were 10 8 cm/s and 10 19 cm -3, respectively, where the Coulomb mean free path is much larger than the size of the interaction region. Simulations of our experimental conditions show that weak Weibel mediated current filamentation and magnetic field generation were likely starting to occur. This paper presents the results from these first Omega experiments. © 2011.
Journal of Applied Physics 109 (2011)
We report on nonequilibrium molecular dynamics simulations of single crystals of copper experiencing rapid shear strain. A model system, with periodic boundary conditions, which includes a single dislocation dipole is subjected to a total shear strain of close to 10 on time-scales ranging from the instantaneous to 50 ps. When the system is strained on a time-scale short compared with a phonon period, the initial total applied shear is purely elastic, and the eventual temperature rise in the system due to the subsequent plastic work can be determined from the initial elastic strain energy. The rate at which this plastic work occurs, and heat is generated, depends on the dislocation velocity, which itself is a function of shear stress. A determination of the stress-dependence of the dislocation velocity allows us to construct a simple analytic model for the temperature rise in the system as a function of strain rate, and this model is found to be in good agreement with the simulations. For the effective dislocation density within the simulations, 7.8 10 11 cm - 2, we find that applying the total shear strain on time-scales of a few tens of picoseconds greatly reduces the final temperature. We discuss these results in the context of the growing interest in producing high pressure, solid-state matter, by quasi-isentropic (rather than shock) compression. © 2011 American Institute of Physics.
IEEE Transactions on Plasma Science 39 (2011) 2822-2823
Measurements of extreme electrostatic and magnetic fields are of interest for the study of high-energy-density plasmas. Results of proton deflectometry of cone-wire targets that are of interest to fast-ignition inertial confinement fusion are presented. © 2006 IEEE.
IEEE Transactions on Plasma Science 39 (2011) 2616-2617
The proton probing technique is used to image quasi-static electromagnetic fields present in the wake of a high-intensity short-pulse laser propagating through an underdense plasma. Bubblelike field structures form along the channel filaments and expand in time. © 2006 IEEE.
INTERNATIONAL TOPICAL CONFERENCE ON PLASMA SCIENCE: STRONGLY COUPLED ULTRA-COLD AND QUANTUM PLASMAS 1421 (2011)