Publications by Gianluca Gregori

Comparison between x-ray scattering and velocity-interferometry measurements from shocked liquid deuterium

Physical Review E - Statistical, Nonlinear, and Soft Matter Physics 87 (2013)

K Falk, BJB Crowley, CD Murphy, JS Wark, G Gregori, SP Regan, SX Hu, PB Radha, J Vorberger, DO Gericke, SH Glenzer, AP Jephcoat

The equation of state of light elements is essential to understand the structure of Jovian planets and inertial confinement fusion research. The Omega laser was used to drive a planar shock wave in the cryogenically cooled deuterium, creating warm dense matter conditions. X-ray scattering was used to determine the spectrum near the boundary of the collective and noncollective scattering regimes using a narrow band x-ray source in backscattering geometry. Our scattering spectra are thus sensitive to the individual electron motion as well as the collective plasma behavior and provide a measurement of the electron density, temperature, and ionization state. Our data are consistent with velocity-interferometry measurements previously taken on the same shocked deuterium conditions and presented by K. Falk. This work presents a comparison of the two diagnostic systems and offers a detailed discussion of challenges encountered. ©2013 American Physical Society.

Simulation of X-ray scattering diagnostics in multi-dimensional plasma

High Energy Density Physics 9 (2013) 510-515

I Golovkin, JJ MacFarlane, P Woodruff, I Hall, G Gregori, J Bailey, E Harding, T Ao, S Glenzer

X-ray scattering is a powerful diagnostic technique that has been used in a variety of experimental settings to determine the temperature, density, and ionization state of warm dense matter. In order to maximize the intensity of the scattered signal, the x-ray source is often placed in close proximity to the target plasma. Therefore, the interpretation of the experimental data can become complicated by the fact that the detector records photons scattered at different angles from points within the plasma volume. In addition, the target plasma that is scattering the x-rays can have significant temperature and density gradients. To address these issues, we have developed the capability to simulate x-ray scattering for realistic experimental configurations where the effects of plasma non-uniformities and a range of x-ray scattering angles are included. We will discuss the implementation details and show results relevant to previous and ongoing experimental investigations. © 2013 Elsevier B.V.

Modeling HEDLA magnetic field generation experiments on laser facilities

High Energy Density Physics 9 (2013) 172-177

M Fatenejad, N Flocke, D Lamb, D Lee, A Scopatz, P Tzeferacos, K Weide, AR Bell, G Gregori, J Meinecke, CD Murphy, A Ravasio, B Reville, M Koenig, JR Marques, A Pelka, R Yurchak, H-S Park, B Remington, A Benuzzi-Mounaix, F Miniati, RP Drake, C Krauland, R Young, R Crowston, N Woolsey

The Flash Center is engaged in a collaboration to simulate laser driven experiments aimed at understanding the generation and amplification of cosmological magnetic fields using the FLASH code. In these experiments a laser illuminates a solid plastic or graphite target launching an asymmetric blast wave into a chamber which contains either Helium or Argon at millibar pressures. Induction coils placed several centimeters away from the target detect large scale magnetic fields on the order of tens to hundreds of Gauss. The time dependence of the magnetic field is consistent with generation via the Biermann battery mechanism near the blast wave. Attempts to perform simulations of these experiments using the FLASH code have uncovered previously unreported numerical difficulties in modeling the Biermann battery mechanism near shock waves which can lead to the production of large non-physical magnetic fields. We report on these difficulties and offer a potential solution. © 2012 Elsevier B.V.

Diffusive shock acceleration at laser-driven shocks: Studying cosmic-ray accelerators in the laboratory

New Journal of Physics 15 (2013)

B Reville, AR Bell, G Gregori

The non-thermal particle spectra responsible for the emission from many astrophysical systems are thought to originate from shocks via a first order Fermi process otherwise known as diffusive shock acceleration. The same mechanism is also widely believed to be responsible for the production of high energy cosmic rays. With the growing interest in collisionless shock physics in laser produced plasmas, the possibility of reproducing and detecting shock acceleration in controlled laboratory experiments should be considered. The various experimental constraints that must be satisfied are reviewed. It is demonstrated that several currently operating laser facilities may fulfil the necessary criteria to confirm the occurrence of diffusive shock acceleration of electrons at laser produced shocks. Successful reproduction of Fermi acceleration in the laboratory could open a range of possibilities, providing insight into the complex plasma processes that occur near astrophysical sources of cosmic rays. © IOP Publishing and Deutsche Physikalische Gesellschaft.

Orbital-free density-functional theory simulations of the dynamic structure factor of warm dense aluminum

Physical Review Letters 111 (2013)

TG White, S Richardson, BJB Crowley, G Gregori, LK Pattison, JWO Harris

Here, we report orbital-free density-functional theory (OF DFT) molecular dynamics simulations of the dynamic ion structure factor of warm solid density aluminum at T=0.5 eV and T=5 eV. We validate the OF DFT method in the warm dense matter regime through comparison of the static and thermodynamic properties with the more complete Kohn-Sham DFT. This extension of OF DFT to dynamic properties indicates that previously used models based on classical molecular dynamics may be inadequate to capture fully the low frequency dynamics of the response function. © 2013 American Physical Society.

Radiative shocks produced from spherical cryogenic implosions at the National Ignition Facility

Physics of Plasmas 20 (2013)

A Pak, L Divol, S Weber, J Atherton, R Bennedetti, DK Bradley, D Callahan, DT Casey, E Dewald, T Döppner, MJ Edwards, S Glenn, D Hicks, WW Hsing, N Izumi, OS Jones, SF Khan, J Lindl, OL Landen, S Le Pape, T Ma, A Macphee, BJ Macgowan, AJ Mackinnon, NB Meezan, JD Moody, JE Ralph, HF Robey, H-S Park, BA Remington, JS Ross, R Tommasini, RPJ Town, V Smalyuk, SH Glenzer, EI Moses, G Gregori, JA Frenje, MG Johnson, GP Grim, JL Kline, GA Kyrala, JD Kilkenny, L Masse, RE Olson

Spherically expanding radiative shock waves have been observed from inertially confined implosion experiments at the National Ignition Facility. In these experiments, a spherical fusion target, initially 2 mm in diameter, is compressed via the pressure induced from the ablation of the outer target surface. At the peak compression of the capsule, x-ray and nuclear diagnostics indicate the formation of a central core, with a radius and ion temperature of ∼20 μm and ∼ 2 keV, respectively. This central core is surrounded by a cooler compressed shell of deuterium-tritium fuel that has an outer radius of ∼40 μm and a density of >500 g/cm. Using inputs from multiple diagnostics, the peak pressure of the compressed core has been inferred to be of order 100 Gbar for the implosions discussed here. The shock front, initially located at the interface between the high pressure compressed fuel shell and surrounding in-falling low pressure ablator plasma, begins to propagate outwards after peak compression has been reached. Approximately 200 ps after peak compression, a ring of x-ray emission created by the limb-brightening of a spherical shell of shock-heated matter is observed to appear at a radius of ∼100 μm. Hydrodynamic simulations, which model the experiment and include radiation transport, indicate that the sudden appearance of this emission occurs as the post-shock material temperature increases and upstream density decreases, over a scale length of ∼10 μm, as the shock propagates into the lower density (∼1 g/cc), hot (∼250 eV) plasma that exists at the ablation front. The expansion of the shock-heated matter is temporally and spatially resolved and indicates a shock expansion velocity of ∼300 km/s in the laboratory frame. The magnitude and temporal evolution of the luminosity produced from the shock-heated matter was measured at photon energies between 5.9 and 12.4 keV. The observed radial shock expansion, as well as the magnitude and temporal evolution of the luminosity from the shock-heated matter, is consistent with 1-D radiation hydrodynamic simulations. Analytic estimates indicate that the radiation energy flux from the shock-heated matter is of the same order as the in-flowing material energy flux, and suggests that this radiation energy flux modifies the shock front structure. Simulations support these estimates and show the formation of a radiative shock, with a precursor that raises the temperature ahead of the shock front, a sharp μ m-scale thick spike in temperature at the shock front, followed by a post-shock cooling layer. © 2013 AIP Publishing LLC.

High-power laser experiments to study collisionless shock generation

EPJ Web of Conferences 59 (2013)

Y Sakawa, Y Kuramitsu, T Morita, T Norimatsu, H Takabe, T Kato, H Tanji, T Ide, T Tsubouchi, K Nishio, M Kuwada, H Ide, C Gregory, N Woolsey, K Schaar, C Murphy, G Gregori, A Diziere, A Pelka, M Koenig, S Wang, Q Dong, Y Li, H-S Park, S Ross, N Kugland, D Ryutov, B Remington, A Spitkovsky, D Froula

A collisionless Weibel-instability mediated shock in a self-generated magnetic field is studied using two-dimensional particle-in-cell simulation [Kato and Takabe, Astophys. J. Lett. 681, L93 (2008)]. It is predicted that the generation of the Weibel shock requires to use NIF-class high-power laser system. Collisionless electrostatic shocks are produced in counter-streaming plasmas using Gekko XII laser system [Kuramitsu et al., Phys. Rev. Lett. 106, 175002 (2011)]. A NIF facility time proposal is approved to study the formation of the collisionless Weibel shock. OMEGA and OMEGA EP experiments have been started to study the plasma conditions of counter-streaming plasmas required for the NIF experiment using Thomson scattering and to develop proton radiography diagnostics. © Owned by the authors, published by EDP Sciences, 2013.

Laboratory experiments on plasma jets in a magnetic field using high-power lasers

EPJ Web of Conferences 59 (2013)

K Nishio, M Kuwada, Y Sakawa, Y Kuramitsu, T Morita, M Koga, T Kato, T Norimatsu, H Takabe, T Ide, C Gregory, N Woolsey, C Murphy, G Gregori, K Schaar, A Diziere, M Koenig, A Pelka, S Wang, Q Dong, Y Li

The experiments to simulate astrophysical jet generation are performed using Gekko XII (GXII) HIPER laser system at the Institute of Laser Engineering. In the experiments a fast plasma flow generated by shooting a CH plane (10 μm thickness) is observed at the rear side of the plane. By separating the focal spot of the main beams, a non-uniform plasma is generated. The non-uniform plasma flow in an external magnetic field (0.2∼0.3 T) perpendicular to the plasma is more collimated than that without the external magnetic field. The plasma β, the ratio between the plasma and magnetic pressure, is ≠1, and the magnetic Reynolds number is ∼150 in the collimated plasma. It is considered that the magnetic field is distorted by the plasma flow and enhances the jet collimation. © Owned by the authors, published by EDP Sciences, 2013.

Simulation of laser-driven, ablated plasma flows in collisionless shock experiments on OMEGA and the NIF

High Energy Density Physics 9 (2013) 192-197

MJ Grosskopf, RP Drake, CC Kuranz, EM Rutter, JS Ross, NL Kugland, C Plechaty, BA Remington, H-S Park, A Spitkovsky, L Gargate, G Gregori, A Bell, CD Murphy, J Meinecke, B Reville, Y Sakawa, Y Kuramitsu, H Takabe, DH Froula, G Fiksel, F Miniati, M Koenig, A Ravasio, E Liang, W Fu, N Woolsey

Experiments investigating the physics of interpenetrating, collisionless, ablated plasma flows have become an important area of research in the high-energy-density field. In order to evaluate the feasibility of designing experiments that will generate a collisionless shock mediated by the Weibel instability on the National Ignition Facility (NIF) laser, computer simulations using the Center for Radiative Shock Hydrodynamics (CRASH) radiation-hydrodynamics model have been carried out. This paper reports assessment of whether the experiment can reach the required scale size while maintaining the low interflow collisionality necessary for the collisionless shock to form. Comparison of simulation results with data from Omega experiments shows the ability of the CRASH code to model these ablated systems. The combined results indicate that experiments on the NIF are capable of reaching the regimes necessary for the formation of a collisionless shock in a laboratory experiment. © 2013.

High Mach-number collisionless shock driven by a laser with an external magnetic field

EPJ Web of Conferences 59 (2013)

T Morita, Y Sakawa, Y Kuramitsu, T Norimatsu, H Takabe, T Ide, K Tsubouchi, A Nishida, K Nishio, M Kuwada, H Ide, H Yoneda, T Namiki, K Tomita, K Nakayama, K Inoue, K Uchino, M Nakatsutsumi, A Pelka, M Koenig, Q Dong, D Yuan, G Gregori

Collisionless shocks are produced in counter-streaming plasmas with an external magnetic field. The shocks are generated due to an electrostatic field generated in counter-streaming laser-irradiated plasmas, as reported previously in a series of experiments without an external magnetic field [T. Morita et al., Phys. Plasmas, 17, 122702 (2010), Kuramitsu et al., Phys. Rev. Lett., 106, 175002 (2011)] via laser-irradiation of a double-CH-foil target. A magnetic field is applied to the region between two foils by putting an electro-magnet (∼10 T) perpendicular to the direction of plasma expansion. The generated shocks show different characteristics later in time (t > 20ns). © Owned by the authors, published by EDP Sciences, 2013.

Probing the complex ion structure in liquid carbon at 100 GPa

Physical Review Letters 111 (2013)

D Kraus, W Cayzac, A Ortner, A Otten, F Roth, G Schaumann, D Schumacher, K Siegenthaler, F Wagner, M Roth, J Vorberger, DO Gericke, K Wünsch, V Bagnoud, A Blažević, A Frank, G Gregori

We present the first direct experimental test of the complex ion structure in liquid carbon at pressures around 100 GPa, using spectrally resolved x-ray scattering from shock-compressed graphite samples. Our results confirm the structure predicted by ab initio quantum simulations and demonstrate the importance of chemical bonds at extreme conditions similar to those found in the interiors of giant planets. The evidence presented here thus provides a firmer ground for modeling the evolution and current structure of carbon-bearing icy giants like Neptune, Uranus, and a number of extrasolar planets. © 2013 American Physical Society.

X-ray scattering by many-particle systems

New Journal of Physics 15 (2013)

BJB Crowley, G Gregori

This paper reviews the treatment of high-frequency Thomson scattering in the non-relativistic and near-relativistic regimes with the primary purpose of understanding the nature of the frequency redistribution correction to the differential cross-section. This correction is generally represented by a factor involving the ratio ω α /ω β of the scattered (α) to primary (β) frequencies of the radiation. In some formulae given in the literature, the ratio appears squared, in others it does not. In Compton scattering, the frequency change is generally understood to be due to the recoil of the particle as a result of energy and momentum conservation in the photon-electron system. In this case, the Klein-Nishina formula gives the redistribution factor as . In the case of scattering by a many-particle system, however, the frequency and momentum changes are no longer directly interdependent but depend also upon the properties of the medium, which are encoded in the dynamic structure factor. We show that the redistribution factor explicit in the quantum cross-section (that seen by a photon) is ω α /ω β, which is not squared. Formulae for the many-body cross-section given in the literature, in which the factor is squared, can often be attributed to a different (classical) definition of the cross-section, though not all authors are explicit about which definition they are using. What is shown not to be true is that the structure factor simply gives the ratio of the many-electron to one-electron differential cross-sections, as is sometimes supposed. Mixing up the cross-section definitions can lead to errors when describing x-ray scattering. We illustrate the nature of the discrepancy by deriving the energy-integrated angular distributions, with first-order relativistic corrections, for classical and quantum scattering measurements, as well as the radiative opacity for photon diffusion in a Thomson-scattering medium, which is generally considered to be governed by quantum processes. © IOP Publishing and Deutsche Physikalische Gesellschaft.

Visualizing electromagnetic fields in laser-produced counter-streaming plasma experiments for collisionless shock laboratory astrophysics

Physics of Plasmas 20 (2013)

NL Kugland, JS Ross, SH Glenzer, C Huntington, MC Levy, D Martinez, C Plechaty, BA Remington, DD Ryutov, H-S Park, P-Y Chang, G Fiksel, DH Froula, RP Drake, M Grosskopf, C Kuranz, G Gregori, J Meinecke, B Reville, M Koenig, A Pelka, A Ravasio, Y Kuramitsu, T Morita, Y Sakawa, H Takabe, E Liang, F Miniati, R Presura, A Spitkovsky

Collisionless shocks are often observed in fast-moving astrophysical plasmas, formed by non-classical viscosity that is believed to originate from collective electromagnetic fields driven by kinetic plasma instabilities. However, the development of small-scale plasma processes into large-scale structures, such as a collisionless shock, is not well understood. It is also unknown to what extent collisionless shocks contain macroscopic fields with a long coherence length. For these reasons, it is valuable to explore collisionless shock formation, including the growth and self-organization of fields, in laboratory plasmas. The experimental results presented here show at a glance with proton imaging how macroscopic fields can emerge from a system of supersonic counter-streaming plasmas produced at the OMEGA EP laser. Interpretation of these results, plans for additional measurements, and the difficulty of achieving truly collisionless conditions are discussed. Future experiments at the National Ignition Facility are expected to create fully formed collisionless shocks in plasmas with no pre-imposed magnetic field. © 2013 AIP Publishing LLC.

X-ray scattering from warm dense iron

High Energy Density Physics 9 (2013) 573-577

S White, G Nersisyan, B Kettle, TWJ Dzelzainis, K McKeever, CLS Lewis, D Riley, A Otten, K Siegenthaler, D Kraus, M Roth, T White, G Gregori, DO Gericke, R Baggott, DA Chapman, K Wünsch, J Vorberger

We have carried out X-ray scattering experiments on iron foil samples that have been compressed and heated using laser-driven shocks created with the VULCAN laser system at the Rutherford-Appleton Laboratory. This is the highest Z element studied in such experiments so far and the first time scattering from warm dense iron has been reported. Because of the importance of iron in telluric planets, the work is relevant to studies of warm dense matter in planetary interiors. We report scattering results as well as shock breakout results that, in conjunction with hydrodynamic simulations, suggest the target has been compressed to a molten state at several 100GPa pressure. Initial comparison with modelling suggests more work is needed to understand the structure factor of warm dense iron. © 2013.

FLASH hydrodynamic simulations of experiments to explore the generation of cosmological magnetic fields

High Energy Density Physics 9 (2013) 75-81

A Scopatz, M Fatenejad, N Flocke, DQ Lamb, D Lee, P Tzeferacos, K Weide, G Gregori, J Meinecke, M Koenig, A Ravasio, R Yurchak

We report the results of FLASH hydrodynamic simulations of the experiments conducted by the University of Oxford High Energy Density Laboratory Astrophysics group and its collaborators at the Laboratoire pour l'Utilisation de Lasers Intenses (LULI). In these experiments, a long-pulse laser illuminates a target in a chamber filled with Argon gas, producing shock waves that generate magnetic fields via the Biermann battery mechanism. The simulations show that the result of the laser illuminating the target is a series of complex hydrodynamic phenomena. © 2012 Elsevier B.V.

FLASH magnetohydrodynamic simulations of shock-generated magnetic field experiments

High Energy Density Physics 8 (2012) 322-328

P Tzeferacos, M Fatenejad, N Flocke, DQ Lamb, D Lee, A Scopatz, K Weide, G Gregori, J Meinecke

We report the results of benchmark FLASH magnetohydrodynamic (MHD) simulations of experiments conducted by the University of Oxford High Energy Density Laboratory Astrophysics group and its collaborators at the Laboratoire pour l'Utilisation des Lasers Intenses (LULI). In these experiments, a long-pulse laser illuminates a target in a chamber filled with Argon gas, producing shock waves that generate magnetic fields via the Biermann battery mechanism. We first outline the implementation of 2D cylindrical geometry in the unsplit MHD solver in FLASH and present results of verification tests. We then describe the results of benchmark 2D cylindrical MHD simulations of the LULI experiments using FLASH that explore the impact of external fields along with the possibility of magnetic field amplification by turbulence that is associated with the shock waves and that is induced by a grid placed in the gas-filled chamber. © 2012 Elsevier B.V.

Studying astrophysical collisionless shocks with counterstreaming plasmas from high power lasers

High Energy Density Physics 8 (2012) 38-45

H-S Park, DD Ryutov, JS Ross, NL Kugland, SH Glenzer, C Plechaty, SM Pollaine, BA Remington, A Spitkovsky, L Gargate, G Gregori, A Bell, C Murphy, Y Sakawa, Y Kuramitsu, T Morita, H Takabe, DH Froula, G Fiksel, F Miniati, M Koenig, A Ravasio, A Pelka, E Liang, N Woolsey, CC Kuranz, RP Drake, MJ Grosskopf

Collisions of high Mach number flows occur frequently in astrophysics, and the resulting shock waves are responsible for the properties of many astrophysical phenomena, such as supernova remnants, Gamma Ray Bursts and jets from Active Galactic Nuclei. Because of the low density of astrophysical plasmas, the mean free path due to Coulomb collisions is typically very large. Therefore, most shock waves in astrophysics are "collisionless", since they form due to plasma instabilities and self-generated magnetic fields. Laboratory experiments at the laser facilities can achieve the conditions necessary for the formation of collisionless shocks, and will provide a unique avenue for studying the nonlinear physics of collisionless shock waves. We are performing a series of experiments at the Omega and Omega-EP lasers, in Rochester, NY, with the goal of generating collisionless shock conditions by the collision of two high-speed plasma flows resulting from laser ablation of solid targets using ∼10 W/cm laser irradiation. The experiments will aim to answer several questions of relevance to collisionless shock physics: the importance of the electromagnetic filamentation (Weibel) instabilities in shock formation, the self-generation of magnetic fields in shocks, the influence of external magnetic fields on shock formation, and the signatures of particle acceleration in shocks. Our first experiments using Thomson scattering diagnostics studied the plasma state from a single foil and from double foils whose flows collide "head-on" Our data showed that the flow velocity and electron density were 10 cm/s and 10 cm , respectively, where the Coulomb mean free path is much larger than the size of the interaction region. Simulations of our experimental conditions show that weak Weibel mediated current filamentation and magnetic field generation were likely starting to occur. This paper presents the results from these first Omega experiments. © 2011.

Testing quantum mechanics in non-Minkowski space-time with high power lasers and 4 th generation light sources

Scientific Reports 2 (2012)

BJB Crowley, CD Murphy, JS Wark, G Gregori, R Bingham, PA Norreys, RG Evans, SJ Rose, DO Gericke, OL Landen, T Tschentscher, CH-T Wang

A common misperception of quantum gravity is that it requires accessing energies up to the Planck scale of 10 GeV, which is unattainable from any conceivable particle collider. Thanks to the development of ultra-high intensity optical lasers, very large accelerations can be now the reached at their focal spot, thus mimicking, by virtue of the equivalence principle, a non Minkowski space-time. Here we derive a semiclassical extension of quantum mechanics that applies to different metrics, but under the assumption of weak gravity. We use our results to show that Thomson scattering of photons by uniformly accelerated electrons predicts an observable effect depending upon acceleration and local metric. In the laboratory frame, a broadening of the Thomson scattered x ray light from a fourth generation light source can be used to detect the modification of the metric associated to electrons accelerated in the field of a high power optical laser.

Plasma switch as a temporal overlap tool for pump-probe experiments at FEL facilities

Journal of Instrumentation 7 (2012)

M Harmand, S Düsterer, T Laarmann, A Przystawik, H Redlin, M Schulz, F Tavella, S Toleikis, D Murphy, D Brown, G Gregori, T White, M Cammarata, D Fritz, J Lee, H Lemke, T Döppner, H Glenzer, E Förster, V Hilbert, U Zastrau, J Gaudin, T Tschentscher, S Göde, K-H Meiwes-Broer, S Skruszewicz, D Hochhaus, P Neumayer, E Galtier, A Moinard

We have developed an easy-to-use and reliable timing tool to determine the arrival time of an optical laser and a free electron laser (FEL) pulses within the jitter limitation. This timing tool can be used from XUV to X-rays and exploits high FELs intensities. It uses a shadowgraph technique where we optically (at 800 nm) image a plasma created by an intense XUV or X-ray FEL pulse on a transparent sample (glass slide) directly placed at the pump - probe sample position. It is based on the physical principle that the optical properties of the material are drastically changed when its free electron density reaches the critical density. At this point the excited glass sample becomes opaque to the optical laser pulse. The ultra-short and intense XUV or X-ray FEL pulse ensures that a critical electron density can be reached via photoionization and subsequent collisional ionization within the XUV or X-ray FEL pulse duration or even faster. This technique allows to determine the relative arrival time between the optical laser and the FEL pulses in only few single shots with an accuracy mainly limited by the optical laser pulse duration and the jitter between the FEL and the optical laser. Considering the major interest in pump-probe experiments at FEL facilities in general, such a femtosecond resolution timing tool is of utmost importance. © 2012 IOP Publishing Ltd and Sissa Medialab srl.

X-ray Thomson scattering on shocked graphite

High Energy Density Physics 8 (2012) 46-49

D Kraus, A Otten, A Frank, A Ortner, G Schaumann, F Wagner, M Roth, V Bagnoud, A Blažević, DO Gericke, D Schumacher, J Vorberger, K Wünsch, G Gregori

We present measurements of the changes in the microscopic structure of graphite in a laser-driven shock experiment with X-ray scattering. Laser radiation with intensities of ∼2 × 10 W/cm compressed the carbon samples by a factor of two reaching pressures of ∼90 GPa. Due to the change of the crystalline structure the scattered signals of the probe radiation were modified significantly in intensity and spectral composition compared to the scattering on cold samples. It is shown that the elastic scattering on tightly bound electrons increases strongly due to the phase transition whereas the inelastic scattering on weakly bound electrons remains nearly unchanged for the chosen geometry. © 2011 Elsevier B.V.